Electronic Structure of Charge- and Spin-Controlled Sr1-(x+y)Lax+yTi1- xCrxO3

Physical Review Letters Volume 96 Issue 6 Page 067203-1-067203-4 published_at 2006-02-14
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Title ( eng )
Electronic Structure of Charge- and Spin-Controlled Sr1-(x+y)Lax+yTi1- xCrxO3
Creator
Yamakawa K.
Saitoh Tomohiko
Inaba Jungo
Katsufuji Takuro
Higashiguchi Mitsuharu
Source Title
Physical Review Letters
Volume 96
Issue 6
Start Page 067203-1
End Page 067203-4
Abstract
We present the electronic structure of Sr1-(x+y)Lax+yTi1-xCrxO3 investigated by high-resolution photoemission spectroscopy. In the vicinity of the Fermi level, it was found that the electronic structure was composed of a Cr 3d local state with the t2g3 configuration and a Ti 3d itinerant state. The energy levels of these Cr and Ti 3d states are well interpreted by the difference of the charge-transfer energy of both ions. The spectral weight of the Cr 3d state is completely proportional to the spin concentration x irrespective of the carrier concentration y, indicating that the spin density can be controlled by x as desired. In contrast, the spectral weight of the Ti 3d state is not proportional to y, depending on the amount of Cr doping.
Keywords
strontium compounds
lanthanum compounds
band structure
photoelectron spectra
carrier density
localised states
charge transfer states
Language
eng
Resource Type journal article
Publisher
American Physical Society
Date of Issued 2006-02-14
Rights
Copyright (c) 2006 The American Physical Society.
Publish Type Version of Record
Access Rights open access
Source Identifier
[ISSN] 0031-9007
[DOI] 10.1103/PhysRevLett.96.067203
[NCID] AA00773679
[DOI] http://dx.doi.org/10.1103/PhysRevLett.96.067203