Antiferroquadrupole order and magnetic field induced octupole in CeB6
PhysRevB.85.174417.pdf 1.16 MB
We have studied the antiferroquadrupole ordered phase of CeB6 in magnetic fields by resonant x-ray diffraction. By analyzing the significant change in the energy spectrum on reversing the field direction along [1̅ 1 0], we have deduced field dependencies of the antiferro components of magnetic dipole, electric quadrupole, and magnetic octupole moments which are simultaneously induced in the Ce 4f orbital with a propagation vector (1/2,1/2,1/2). The data treatments are based on theoretically calculated spectral functions. The existence of the field-induced octupole is also concluded for other field directions. We also show direct evidence for the formation of a linear-combination-type antiferroquadrupole order parameter in magnetic fields, which is expressed as 〈αOyz+βOzx+γOxy〉 and changes continuously with the field direction (α,β,γ). A possibility of observing the quadrupolar fluctuation is also pointed out.
Physical Review B
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American Physical Society
(c) 2012 American Physical Society
Graduate School of Advanced Sciences of Matter